Trying to install Ember-CLI, unable to find module 'Chalk'

That means npm was installed with admin rights (EACCES means that it can’t add that package to your modules folder because it’s admin-only). Try following these instructions for uninstalling.

EDIT: From that file path, I’m guessing you’re on Windows? I’m not sure how you installed node, but you might give these instructions a shot. As for reinstalling, the installer on the main site is probably your best bet.